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- W1993673353 abstract "Abstract Three new complexes Ln(BDC)1.5(DEF) [Ln = La(1), Ce(2), Nd(3); H2BDC = 1,4-benzenedicarboxylic acid; DEF = N,N-diethylformamide] have been solvothermally synthesized and characterized by single-crystal X-ray diffraction. Complexes 1–3 are isostructural and crystallize in triclinic space group P 1 ¯ . They display three-dimensional frameworks and 18.7986 A × 11.3230 A rhombic channels along the a axis without interpenetration. Two eight-coordinated metal centers are connected with two dimonodentate BDC groups and two chelating/bridging bidentate BDC groups to give a paddle-wheel building block. The building blocks are connected through two carboxyl groups to lead to a one-dimensional infinite inorganic chain (–M–O–C–O–M–) along the [1 0 0] direction. Thermogravimetric analyses (TGA) and X-ray powder diffraction (XPRD) were determined for the three complexes. An observed intense blue luminescence with an emission band peaking at 372 nm for them may result from ligand-to-metal charge transfer (LMCT). Variable-temperature magnetic susceptibility of 2 and 3 was investigated and found deviated from the Curie–Weiss law." @default.
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- W1993673353 date "2008-05-01" @default.
- W1993673353 modified "2023-09-24" @default.
- W1993673353 title "Syntheses, structures and properties of novel 3D lanthanide metal-organic frameworks with paddle-wheel building blocks" @default.
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- W1993673353 doi "https://doi.org/10.1016/j.ica.2007.10.043" @default.
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