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• W1993847178 abstract "Density functional theory (DFT) is employed to investigate the initial growth mechanism of atomic layer deposition (ALD) of ZnO on the hydroxylated silicon surfaces. Both the diethylzinc (DEZn) and the H2O half-reactions proceed through an analogous trapping-mediated mechanism. By comparison of the reactions on silicon surfaces with single and double hydroxyl sites, we find that the existence of neighboring hydroxyl can facilitate the adsorption of DEZn and lower the activation barrier. Also, we find that it is both thermodynamically and kinetically more favorable for the reactions on silicon surfaces with double hydroxyl sites. In addition, calculations show that the DEZn half-reaction is more favorable as compared to the H2O half-reaction." @default.
• W1993847178 created "2016-06-24" @default.
• W1993847178 creator A5049958305 @default.
• W1993847178 date "2009-03-01" @default.
• W1993847178 modified "2023-09-23" @default.
• W1993847178 title "Initial growth mechanism of atomic layer deposition of ZnO on the hydroxylated Si(100)-2×1: A density functional theory study" @default.
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• W1993847178 doi "https://doi.org/10.1016/j.apsusc.2008.12.077" @default.
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