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- W1993896454 abstract "The Flory−Huggins equation was modified and applied to low-weight nonelectrolyte solutions. The following modifications have been made: (1) the Wilson expressions for the local compositions were changed to account for the dependence of the interaction energy parameter between molecules of different types on the mole fraction (a linear dependence was assumed); (2) the above change led to a composition dependent Flory−Huggins interaction parameter χ; (3) the bulk volume fractions in the Flory−Huggins equation have been replaced with local volume fractions. The new equations have been tested for 35 binary alcohol−water vapor−liquid equilibria sets. It has been shown that the new equations represent in most cases better the vapor−liquid equilibria data than the Wilson and the NRTL equations. The capability of the new equations to predict the activity coefficients at infinite dilution from vapor−liquid equlibrium data at finite composition was also tested. It was found that the new equations provide better agreement with the experimental activity coefficients at infinite dilution than the Wilson and the NRTL equations do." @default.
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- W1993896454 date "1999-09-03" @default.
- W1993896454 modified "2023-10-16" @default.
- W1993896454 title "Modified Local Composition and Flory−Huggins Equations for Nonelectrolyte Solutions" @default.
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- W1993896454 doi "https://doi.org/10.1021/ie990230q" @default.
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