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• W1994126720 abstract "Since their first utilisation in 1958 for the synthesis of graft copolymers, macromonomers have raised increasing interest because of their ability to provide an easy access to a large number of (co)polymers of different chemical natures and various controlled topologies (comb-like, bottlebrush, star-like, graft copolymers...) exhibiting very different solution or solid-state properties compared to their linear homologues. During the first decades, the (co)polymerisation of macromonomers was based on poorly controlled free radical polymerisations. Therefore, it was difficult to obtain polymers in a controlled manner. With the appearance of Ring Opening Metathesis Polymerisation (ROMP) or of new free radical processes such as Atom Transfer Radical Polymerisation (ATRP) that allow control of molar masses, and of Ziegler–Natta-type polymerisation that allows control of the tacticity of the polymacromonomer backbone, these processes have been increasingly utilised for macromonomer (co)polymerisations. In this paper, a review of the results published in the literature regarding the homopolymerisation of macromonomers in the presence of transition metal is presented. Depuis leur première utilisation en 1958 pour la synthèse de copolymères greffés, l’intérêt suscité par les macromonomères n’a cessé d’augmenter, car ils permettent un accès aisé à des structures nouvelles (peignes, goupillons, étoiles, copolymères greffés...) ayant des propriétés en solution ou à l’état solide très différentes de celles de leurs homologues linéaires. Pendant de nombreuses années, leur (co)polymérisation a surtout été étudiée par voie radicalaire. Néanmoins, l’obtention de polymacromonomères de manière contrôlée s’est avérée difficile par cette technique. La ROMP (polymérisation par métathèse par ouverture de cycle) ou l’ATRP (polymérisation radicalaire par transfert d’atome) permettant de contrôler la masse molaire des polymacromonomères et les polymérisations de type Ziegler–Natta conduisant à des polymacromonomères dont le squelette est stéréorégulier, ces procédés ont été utilisés plus récemment pour la (co)polymérisation des macromonomères. Dans cet article, nous faisons le point sur les travaux publiés dans la littérature concernant l’homopolymérisation de macromonomères par des techniques de polymérisation faisant appel à des métaux de transition." @default.
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• W1994126720 date "2002-04-01" @default.
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• W1994126720 title "Transition metal-based homopolymerisation of macromonomers" @default.
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• W1994126720 doi "https://doi.org/10.1016/s1631-0748(02)01369-3" @default.
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