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- W1994149170 abstract "The phosphorescent triplet state T1 of p-chloroaniline (PCA) in a p-xylene host, in a neat crystal (n-trap), and in a PCA crystal doped with p-dichlorobenzene (x-trap) has been studied with the aid of phosphorescence spectra, optically detected zero-field magnetic resonance, and T1←S0 absorption spectra at temperatures below 4.2 K. The dynamic properties, particularly the radiative properties, of the individual spin states of T1 are discussed in detail using the emission spectra for each spin state obtained with microwave techniques. For the x-trap system, the emissions from the Ty and Tz sublevels are found to be coincident in contrast to the other two systems. From this observation, it is suggested that the characters of the Ty and Tz states of normal PCA are mixed together in the x-trap.The populating rates for the individual spin states were examined for the PCA crystal systems as a function of the excitation energy, when the excitation was induced by light having wavelengths in the T1←S0 absorption region. The relative populating rates thus obtained are dependent on the excitation energy. Therefore, it is concluded that the spin alignment produced by direct optical pumping from the ground state to the triplet manifold of the crystal is conserved during the vibrational relaxation and energy transfer processes. By using this unique wavelength dependence of the populating rates, the nature of the n- and x-traps is discussed and the vibrational structure of the T1←S0 spectrum is analyzed." @default.
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- W1994149170 date "1976-05-01" @default.
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- W1994149170 title "An Investigation of the Triplet State Dynamics of<i>p</i>-Chloroaniline by Microwave Induced Changes in the Phosphorescence Intensity and by Triplet←Singlet Absorption" @default.
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- W1994149170 doi "https://doi.org/10.1246/bcsj.49.1221" @default.
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