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• W1994168112 endingPage "6039" @default.
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• W1994168112 abstract "X-ray photoelectron spectra and electron-energy-loss spectra (EELS) are presented and interpreted for Pd${mathrm{H}}_{mathrm{ensuremath{sim}}0.8}$ prepared by in situ loading and cleaning of a 10-ensuremath{mu}m foil cooled to 80 K. Hydrogenation induces new states with considerable $d$ character 8 eV in the valence band, a slight narrowing of the valence-band spectrum, and a shift of the Fermi level out of the $d$ manifold of states. In the core-line spectra a +0.17-eV binding-energy shift occurs, the asymmetry is reduced, and a shake-up satellite at 6 eV essentially disappears. In the EELS spectra a 7-eV plasmon loss is attenuated and shifted to 5 eV. During degassing experiments, no significant surface depletion is found, and two different rates occur: For concentrations ${mathrm{H}}_{x}ensuremath{gtrsim}0.65$ atomic fraction hydrogen (($ensuremath{beta}$ phase) an activation energy of 8.1-kcal/mole ${mathrm{H}}_{2}$ is found, while for ${mathrm{H}}_{x}ensuremath{gtrsim}0.65$ (two-phase region) the rate is ${10}^{5}$ slower, but has a similar activation energy of 9.0-kcal/mole ${mathrm{H}}_{2}$. During this time the surface contains both $ensuremath{beta}$ and $ensuremath{alpha}$ phases." @default.
• W1994168112 created "2016-06-24" @default.
• W1994168112 creator A5053630523 @default.
• W1994168112 creator A5071868218 @default.
• W1994168112 date "1982-12-01" @default.
• W1994168112 modified "2023-10-16" @default.
• W1994168112 title "Electronic structure and surface kinetics of palladium hydride studied with x-ray photoelectron spectroscopy and electron-energy-loss spectroscopy" @default.
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• W1994168112 doi "https://doi.org/10.1103/physrevb.26.6030" @default.
• W1994168112 hasPublicationYear "1982" @default.
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