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- W1994405718 abstract "The new generation of secondary organic aerosol (SOA) models that represent gas- and particle-phase chemistry and thermodynamic partitioning using discrete two-dimensional grids (e.g. SOM, 2D-VBS) cannot be efficiently implemented into three-dimensional atmospheric chemical transport models (CTMs) due to the large number of bins (tracers) required. In this study, we introduce a novel mathematical framework, termed the Oxidation State/Volatility Moment Method, that is designed to address these computational burdens so as to allow the new generation of SOA models to be implemented into CTMs. This is accomplished by mapping the two-dimensional grids onto probability distributions that conserve carbon and oxygen mass. Assessment of the Moment Method strengths (speed, carbon and oxygen conservation) and weaknesses (numerical drift) provide valuable insight that can guide future development of SOA modules for atmospheric CTMs." @default.
- W1994405718 created "2016-06-24" @default.
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- W1994405718 date "2014-10-01" @default.
- W1994405718 modified "2023-10-17" @default.
- W1994405718 title "Insight into the numerical challenges of implementing 2-dimensional SOA models in atmospheric chemical transport models" @default.
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- W1994405718 doi "https://doi.org/10.1016/j.atmosenv.2014.07.048" @default.
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