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• W1994405778 abstract "The quantum kinetic chemical reaction model proposed by Bird for the direct simulation Monte Carlo method is based on collision kinetics with no assumed Arrhenius-related parameters. It demonstrates an excellent agreement with the best estimates for thermal reaction rates coefficients and with two-temperature nonequilibrium rate coefficients for high-temperature air reactions. This paper investigates this model further, concentrating on the non-thermal reaction cross sections as a function of collision energy, and compares its predictions with those of the earlier total collision energy model, also by Bird, as well as with available quasi-classical trajectory cross section predictions (this paper also publishes for the first time a table of these computed reaction cross sections). A rarefied hypersonic flow over a cylinder is used to examine the sensitivity of the number of exchange reactions to the differences in the two models under a strongly nonequilibrium velocity distribution." @default.
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• W1994405778 date "2012-04-01" @default.
• W1994405778 modified "2023-10-06" @default.
• W1994405778 title "Reaction cross sections for two direct simulation Monte Carlo models: Accuracy and sensitivity analysis" @default.
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• W1994405778 doi "https://doi.org/10.1063/1.3701379" @default.
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