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• W1994428591 abstract "Sol–gel distributions at high conversions, simulated by computer with spatial constraints on the distribution of chain ends, are reported for end-linked tetrafunctional systems. The composition of the sol is found to be uniquely dependent upon the functionality f of the cross linker: for f=4, it mainly consists of linear monomers and oligomers containing one saturated cross linker. The molecular weight distribution of the sol exhibits a shoulder at the trimer due to the relative abundance of the ‘‘bow-tie’’ molecule. The populations of various types of dangling ends and loop defects in the gel are given and discussed. Our simulations reveal empirically that the single-loop probability varies with the −3/8 power of the molecular weight of the prepolymers. The power-law dependence of the loop formation on chain length of the prepolymers and the nonrandom nature of the cross-linking reaction is discussed." @default.
• W1994428591 created "2016-06-24" @default.
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• W1994428591 date "1984-04-15" @default.
• W1994428591 modified "2023-10-01" @default.
• W1994428591 title "Computer simulation of end-linked elastomers. II. Bulk cured tetrafunctional networks" @default.
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• W1994428591 doi "https://doi.org/10.1063/1.447170" @default.
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