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- W1994516903 abstract "An approximate theory for the interaction of classical radiation with a quantum mechanical molecule is given. The theory is based on the idea that when the field frequency is of the order of the electronic frequency, a separation of the electronic and nuclear motions is possible in the presence, as in the absence, of the field. A weak field is assumed, and time-dependent perturbation theory is used to obtain the amplitudes and cross sections for photodissociation and Raman scattering. The semiclassical coordinate-space (sc) results are shown to correspond to accurate short-time dynamics on the excited Born–Oppenheimer surfaces for nuclear motion. Calculations are performed for ICN using a two-dimensional collinear model." @default.
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- W1994516903 date "1982-03-15" @default.
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- W1994516903 title "Semiclassical theory of radiation interacting with a molecule" @default.
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- W1994516903 doi "https://doi.org/10.1063/1.443346" @default.
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