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• W1994547622 abstract "Setting up the correct functionality with the correct stereochemistry in the ring-A of anthracycline precursors represents a synthetic challenge. The use of d-glucose as a chiral auxiliary either on the silyloxy diene or naphthoquinone-based dienophile to form the ring-A using asymmetric Diels–Alder reactions as developed by the Stoodley group and is the focus of this review. The endo-transition state is described based on a frontier orbital approach and the HOMO–LUMO energy gaps were estimated using semi-empirical (MNDO) calculations with SPARTAN’08. As anthracyclines are used in chemotherapy, some of their associated biochemistry and clinical effectiveness are also briefly introduced." @default.
• W1994547622 created "2016-06-24" @default.
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• W1994547622 date "2013-01-01" @default.
• W1994547622 modified "2023-09-25" @default.
• W1994547622 title "Studies directed towards anthracyclinone syntheses: The use of d-glucose as a chiral auxiliary in asymmetric Diels–Alder reactions" @default.
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• W1994547622 doi "https://doi.org/10.1016/j.jscs.2011.02.019" @default.
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