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• W1995168701 abstract "This work forms part of a study of the extraction equilibria in the quaternary system uranyl nitrate-water-TBP-carbon tetrachloride.In the ternary system CCl4-H2O-TBP two liquid layers occur. From the three binaries that limit this system the pairs TBP-H2O and CCl4-H2O have a miscibility-gap, while the pair TBP -CCl4 is fully miscible.The extremely asymmetric miscibility-gap in the system water-tributyl phosphate (TBP) has given rise to the assumption that a compound with composition H2O · TBP is formed. A number of authors have argued for the existence of this compound, based on spectral evidence. We have measured the freezing point diagram and some solubility data in this system as a function of temperature. From the results we conclude that the compound mentioned does not exist to any appreciable concentration in solutions of water in TBP, although these solutions show an appreciable deviation from ideality. This non-ideal behaviour was investigated by isopiestic vapour pressure measurements. Data on the activity coefficients of water in TBP are given at 25.0°. They are represented by the equationIn f = x2 [1.563 - 1.143 (4 x - 3) + 0.682 (2 x - 1) (6 x - 5)] x being the mole fraction of TBP.Data on vapour pressures and activity coefficients for the binary TBP -CCl4 are given at 25.0°. In the ternary phase diagram the miscibility boundary has been determined at the same temperature." @default.
• W1995168701 created "2016-06-24" @default.
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• W1995168701 date "2010-09-02" @default.
• W1995168701 modified "2023-09-25" @default.
• W1995168701 title "The ternary system: Carbon tetrachloride - water - tributyl phosphate (TBP)" @default.
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• W1995168701 doi "https://doi.org/10.1002/recl.19640830716" @default.
• W1995168701 hasPublicationYear "2010" @default.
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