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• W1995207844 startingPage "4561" @default.
• W1995207844 abstract "Rotationally resolved transitions from the metastable 4sσ a3Σ+u state of Ar2 to the 7pσ 3Σ+g state have been observed by laser excitation spectroscopy in a pulsed corona discharge. Laser induced fluorescence spectra for the 7pσ 3Σ+g←a3Σ+u transition observed near 19 530 cm−1 have led to the first resolved triplet splittings and rotational analyses for Rydberg–Rydberg transitions in Ar2. Analyses for the (0–0), (0–1), (1–0), and (1–1) bands of 7pσ←a are presented here. Bands with v′=2 are observed for this system but exhibit no rotational structure and bands with v′≳2 are not observed, indicating that the predissociation lifetimes of these upper levels fall rapidly for v′≳1. Data presented lead to rotational energies and molecular constants for the a3Σ+u and 7pσ 3Σ+g states, including the effective rotational constant Be which is determined to be 0.1412 cm−1 and 0.1345 cm−1 for the 4sσ a3Σ+u and 7pσ 3Σ+g states, respectively. Results are compared to ab initio and other calculations, and combined with existing data to produce experimental estimates of D0 and De for the a3Σ+u state of 5700±200 cm−1 and 5850±200 cm−1, respectively." @default.
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• W1995207844 date "1994-09-15" @default.
• W1995207844 modified "2023-10-16" @default.
• W1995207844 title "Rotational analysis of the 7<i>p</i>σ 3Σ+<i>g</i>←<i>a</i>3Σ+<i>u</i> system of the Ar2 molecule" @default.
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• W1995207844 doi "https://doi.org/10.1063/1.467443" @default.
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