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• W1995230610 abstract "Single-crystalline thin film of an iridium dioxide polymorph Ir2O4 has been fabricated by the pulsed laser deposition of LixIr2O4 precursor and the subsequent Li-deintercalation using soft chemistry. Ir2O4 crystallizes in a spinel (AB2O4) without A cations in the tetrahedral site, which is isostructural to λ-MnO2. Ir ions form a pyrochlore sublattice, which is known to give rise to a strong geometrical frustration. This Ir spinel was found to be a narrow gap insulator, in remarkable contrast to the metallic ground state of rutile-type IrO2. We argue that an interplay of a strong spin-orbit coupling and a Coulomb repulsion gives rise to an insulating ground state as in a layered perovskite Sr2IrO4." @default.
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• W1995230610 date "2010-05-03" @default.
• W1995230610 modified "2023-09-30" @default.
• W1995230610 title "Epitaxially stabilized iridium spinel oxide without cations in the tetrahedral site" @default.
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• W1995230610 doi "https://doi.org/10.1063/1.3374449" @default.
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