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• W1995360596 abstract "We have studied the capabilities of intense ultrashort chirped pulses for controlling the long range electron transfer in systems strongly coupled to a polar medium. We considered a two state electronic donor/acceptor system, possessing a large difference of permanent dipole moments between donor and acceptor states, with relaxation treated as a diffusion on electronic potential energy surfaces. This relaxation model has enabled us to trace continuously the transition from a coherent population transfer to incoherent one. In addition to the field controlled electron transfer, we take into account a possibility of the direct optical transition between electronic states under study as well. We have introduced the generalized Rabi frequency that enabled us to extend the concepts and ideas of population transfer, developed for optical transitions, to the electron transfer (radiationless process) controlled with strong electromagnetic field. We have shown that it is possible to realize the “radiationless” analogies to π-pulse excitation, adiabatic rapid passage and pump–dump process. We have obtained a physically clear picture of the analogy to the adiabatic rapid passage for the chirped controlled long-range electron transfer by studying vibrationally non-equilibrium populations behavior and careful examination of all the conditions needed for adiabatic rapid passage." @default.
• W1995360596 created "2016-06-24" @default.
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• W1995360596 date "2004-12-01" @default.
• W1995360596 modified "2023-10-09" @default.
• W1995360596 title "Chirped pulse control of long range electron transfer" @default.
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• W1995360596 doi "https://doi.org/10.1016/j.chemphys.2004.07.049" @default.
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