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• W1995633130 abstract "Small-angle x-ray scattering (SAXS) from single-phase melts and solutions of polystyrene-block-polyisoprene (SI) having various degrees of polymerization N and compositions f were analyzed on the basis of Landau-type mean-field theory developed by Leibler. The effective Flory interaction parameter χeff per segment in melts and in semidilute Θ solutions were determined from the mean-field analysis of the SAXS profiles obtained at temperatures higher than TMF, the crossover temperature above which the non-mean-field effects become less significant and the mean-field theory becomes a good approximation. It was found that χeff thus determined depends on N, f, volume fraction of the SI in the solution φp and the interaction parameter χ0 in melt: χeff=φpχ0 and χ0 is a function of f and N; χ0 at a given f is a decreasing function of N and that at a given N is approximately a quadratic function of f with a minimum at f≂1/2." @default.
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• W1995633130 date "1996-05-15" @default.
• W1995633130 modified "2023-10-14" @default.
• W1995633130 title "Order-disorder transition of polystyrene-<i>block</i>-polyisoprene. I. Thermal concentration fluctuations in single-phase melts and solutions and determination of χ as a function of molecular weight and composition" @default.
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• W1995633130 doi "https://doi.org/10.1063/1.471656" @default.
• W1995633130 hasPublicationYear "1996" @default.
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