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- W1996145188 abstract "A systematic investigation of the conceptofpre-organization of nonlinear optical (NLO) active chromophoric groups in calix[4]arene derivatives and the influence on the absolute second-order nonlinear optical coefficients is reported. Several calix[4]arenes were synthesized by modification of the electron-withdrawing groups at the upper rim of the aromatic and extension of the conjugated π system of the pre-organized chromophoric groups. Electrical field induced second harmonic generation (EFISH) experiments showed high μβ(0) values up to 1165·10−48 esu. Compared with the corresponding reference compounds, enhancements of the μβ(0) values varying up to 2.5 times per chromophore were observed which proves the benefit of pre-organization of NLO-active units in a multi-chromophoric system. Another important advantage is that the increase in NLO activity observed for these systems is not accompanied with a shift of the absorption band to longer wavelengths exceeding 20 nm. This makes these calix[4]arene derivatives promising building blocks for the development of stable, NLO-active materials that are suitable for frequency doubling." @default.
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- W1996145188 date "1998-06-01" @default.
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- W1996145188 title "High Hyperpolarizabilities of Donor-π-Acceptor-Functionalized Calix[4]arene Derivatives by Pre-organization of Chromophores" @default.
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- W1996145188 doi "https://doi.org/10.1002/(sici)1099-0690(199806)1998:6<1089::aid-ejoc1089>3.0.co;2-t" @default.
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