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• W1996456507 abstract "A detailed reaction mechanism has been proposed for the full ALD cycle of Si3N4 deposition on the β-Si3N4(0001) surface using bis(diethylamino)silane (BDEAS) or bis(tertiarybutylamino)silane (BTBAS) as a Si precursor with NH3 acting as the nitrogen source. Potential energy landscapes were derived for all elementary steps in the proposed reaction network using a periodic slab surface model in the density functional approximation. Although the dissociative reactivity of BTBAS was slightly better than that of BDEAS, the thermal deposition process was still found to be an inherently high temperature process due to the high activation energies during the dissociative chemisorption of both precursors and the surface re-amination steps. These results underline the need to develop new precursors and alternative nitrogen sources when low temperature thermal silicon nitride films are targeted." @default.
• W1996456507 created "2016-06-24" @default.
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• W1996456507 date "2014-07-22" @default.
• W1996456507 modified "2023-10-16" @default.
• W1996456507 title "Density functional theory study on the full ALD process of silicon nitride thin film deposition via BDEAS or BTBAS and NH₃" @default.
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• W1996456507 doi "https://doi.org/10.1039/c4cp02741h" @default.
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