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- W1996484313 abstract "The adsorption of halogenated acetonitrile (X−CH2C≡N, X = F, Cl, Br) on Si(100)-2×1 has been studied using high-resolution electron energy loss spectroscopy (HREELS), X-ray photoelectron spectroscopy (XPS), and density functional theory (DFT) calculation. Fluoroacetonitrile chemisorbs on the Si(100)-2×1 surface via a C≡N [2 + 2] cycloaddition-like reaction, while chloroacetonitrile is chemically bound to the Si surface through both C≡N [2 + 2] cycloaddition-like and ene-like reactions. However, bromoacetonitrile was found to attach onto the surface exclusively through the ene-like reaction. The different reaction pathways of these halogenated compounds on the Si(100)-2×1 surface demonstrate that the halogen substitution groups play an important role in manipulating the reaction channels of bifunctional molecules, offering a great flexibility in surface reaction of silicon surfaces." @default.
- W1996484313 created "2016-06-24" @default.
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- W1996484313 date "2010-01-22" @default.
- W1996484313 modified "2023-09-28" @default.
- W1996484313 title "Switching from a [2 + 2] Cycloaddition-Like to an Ene-Like Reaction in Covalent Attachment of Halogenated Acetonitrile on Si(100)-2×1: Effect of Halogen Substituent" @default.
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- W1996484313 doi "https://doi.org/10.1021/jp910314p" @default.
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