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• W1996591683 abstract "We report the first in situ boron $K$-edge inelastic x-ray scattering (IXS) spectra for alkali borate glasses (${mathrm{Li}}_{2}{mathrm{B}}_{4}{mathrm{O}}_{7}$) at high pressure up to 30 GPa where pressure-induced coordination transformation from three-coordinated to four-coordinated boron was directly probed. Coordination transformation (reversible upon decompression) begins around 5 GPa and the fraction of four-coordinated boron increases with pressure from about 50% (at 1 atm) to more than 95% (at 30 GPa) with multiple densification mechanisms, evidenced by three distinct pressure ranges for $(d^{[4]}mathrm{B}/dP{)}_{T}$. The lithium $K$-edge IXS spectrum for Li-borate glasses at 5 GPa shows IXS features similar to that at 1 atm, suggesting that the Li environment does not change much with pressure up to 5 GPa. These results provide improved understanding of the structure of low-$z$ glass at high pressure." @default.
• W1996591683 created "2016-06-24" @default.
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• W1996591683 date "2007-03-06" @default.
• W1996591683 modified "2023-10-15" @default.
• W1996591683 title "Structure of Alkali Borate Glasses at High Pressure: B and Li<mml:math xmlns:mml=http://www.w3.org/1998/Math/MathML display=inline><mml:mi>K</mml:mi></mml:math>-Edge Inelastic X-Ray Scattering Study" @default.
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• W1996591683 doi "https://doi.org/10.1103/physrevlett.98.105502" @default.
• W1996591683 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/17358545" @default.
• W1996591683 hasPublicationYear "2007" @default.
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