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• W1996703048 abstract "The energy distribution among rotational levels of NH 3 molecules in a supersonic beam is measured at a position distant from the nozzle by the highly sensitive infrared laser Stark spectroscopic method. A nonequilibrium energy distribution is observed within the rotational degree of freedom. In particular, population inversion is observed on some rotational levels. Computer simulation based on a novel rate-equation model, in which the dipole-dipole interaction, detailed balance, and hard-sphere collisions are assumed, reproduces the observed results well. This model is able to characterize the internal energy distribution of a supersonic beam under various experimental conditions by means of a scaling parameter." @default.
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• W1996703048 date "1992-04-01" @default.
• W1996703048 modified "2023-10-17" @default.
• W1996703048 title "Nonequilibrium Rotational Energy Distribution in NH₃ Supersonic Molecular Beam" @default.
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• W1996703048 doi "https://doi.org/10.1143/jjap.31.1199" @default.
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