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- W1996716992 abstract "A number of examples are given to illustrate the use of computer modeling to elucidate the structures of elastomeric polymer networks, and to provide guidance on controlling network structure to maximize mechanical properties. The first example involves simulations of the gelation process leading to the development of the network structure necessary for a material to exhibit reversible elastomeric properties. The goals here are to characterize the amounts and constitutents of the sol phase, and the structure of the gel phase sufficient for prediction of its mechanical properties. Attempts are also being made to simulate the structure and properties of networks having multimodal distributions of chain lengths, for example to suggest how trimodal distributions might give additional improvements beyond those shown by bimodal networks. Network thermoelasticity can also be elucidated by simulations of the temperature dependence of the unperturbed dimensions of the network chains. Strain-induced crystallization is also being simulated to generate chains having sequence distributions that are representative of various polymerization conditions. The chains are then placed alongside one another to determine matched-sequence runs that could lead to the formation of crystallites. Finally, the long-standing problem of clarifying how fillers reinforce elastomeric materials is being approached using simulations of chains in the vicinity of impenetrable filler particles. In this way it is possible to determine how reinforcement depends on the perturbation of distributions caused by this excluded-volume effect." @default.
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- W1996716992 date "2001-06-01" @default.
- W1996716992 modified "2023-10-14" @default.
- W1996716992 title "Some simulations on elastomers and rubberlike elasticity" @default.
- W1996716992 doi "https://doi.org/10.1002/1521-3900(200106)171:1<1::aid-masy1>3.0.co;2-x" @default.
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