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• W1996838204 abstract "This paper investigates effects of using monodisperse inverse analyses to extract particle-particle and particle-surface potentials from simulated interfacial colloidal fluids of polydisperse attractive particles. Effects of polydispersity are investigated as functions of particle concentration and attractive well depth and range for van der Waals and depletion potentials. Forward Monte Carlo simulations are used to generate particle distribution functions for polydisperse interfacial colloidal fluids from which inverted potentials are obtained using an inverse Ornstein-Zernike analysis and an inverse Monte Carlo simulation method. Attractive potentials are successfully recovered for monodisperse colloidal fluids, but polydispersity that is unaccounted for in inverse analyses produces (1) apparent softening of strong forces, (2) anomalous repulsive and attractive interactions, and (3) aphysical particle overlaps. This investigation provides insights into the role of polydispersity in altering the equilibrium structure and corresponding inverted potentials of attractive colloidal fluids near surfaces. These findings should assist the design and interpretation of optical microscopy experiments involving interfacial colloidal fluids similar to the simulated experiments reported here." @default.
• W1996838204 created "2016-06-24" @default.
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• W1996838204 date "2006-02-03" @default.
• W1996838204 modified "2023-10-16" @default.
• W1996838204 title "Anomalous potentials from inverse analyses of interfacial polydisperse attractive colloidal fluids" @default.
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• W1996838204 doi "https://doi.org/10.1063/1.2162536" @default.
• W1996838204 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/16468906" @default.
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