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- W1997001047 abstract "The first resonance Raman spectra of Cl2O dissolved in CCl4 are reported. The dependence of the resonance Raman spectrum on incident energy is investigated and found to be consistent with the photochemical production of both ClO and ClClO. Both of these photoproducts appear linearly with incident energy at low power, but the scattering intensity of ClO is found to increase quadratically at higher energies. This behavior is proposed to be consistent with photodissociation of Cl2O into ClO and Cl followed by partial geminate recombination of these fragments, resulting in ClClO formation. At higher excitation energies, photodissociation of ClClO is proposed to occur resulting in ClO production. Finally, the photochemical behavior of Cl2O is compared to that of OClO, where geminate recombination does not result in formation of the analogous ClOO isomer. This comparison suggests that although geminate recombination is a characteristic feature of halo-oxide photochemistry in condensed environments, the products formed by recombination are species dependent." @default.
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- W1997001047 date "1999-12-01" @default.
- W1997001047 modified "2023-10-18" @default.
- W1997001047 title "A resonance Raman study of Cl2O photochemistry in solution: evidence for ClClO formation" @default.
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- W1997001047 doi "https://doi.org/10.1016/s1010-6030(99)00181-1" @default.
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