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• W1997261566 abstract "A new scheme for performing high-resolution kinetic energy measurements on single quantum states of NO is described. Laser excitation of the a 4Π(ν=13–15) and b 4Σ−(ν=3)←X 2Π(ν=0) spin-forbidden bands has been used to produce NO a 4Π, either by direct excitation or after excitation to NO b 4Σ− followed by b→a emission. The sensitivity is compared to previous experiments on CO, employing the forbidden Cameron system. In the course of these experiments, three previously unknown vibronic levels of the a 4Π state were observed for which high precision molecular constants have been obtained. The derived molecular constants have been used to construct a chemically accurate RKR potential for the a 4Π state to within 0.2 eV of the dissociation limit. In addition, the electric dipole moments for the a 4Π(ν=13–14) levels have been determined. By comparing the experimental results with two ab initio calculations, the polarity of the dipole moment of the a 4Π state at equilibrium separation could be determined. A set of supplementary molecular beam laser-induced fluorescence studies on the b 4Σ−(ν=3)←X 2Π(ν=0) band were also carried out. These allowed the fluorescence lifetime of b 4Σ−(ν=3) state to be obtained under collision-free conditions and the electronic origin of the quartet manifold to be determined within 0.03 cm−1." @default.
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• W1997261566 date "1995-11-08" @default.
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• W1997261566 title "The spin-forbidden <i>a</i> 4Π(ν=13–15) and <i>b</i> 4Σ−(ν=3)←<i>X</i> 2Π(ν=0) bands of nitric oxide: A new scheme for quantum state-specific high-resolution kinetic energy measurements" @default.
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• W1997261566 doi "https://doi.org/10.1063/1.470292" @default.
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