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- W1997627838 abstract "The core binding energies of N1s and S2s in cis-1,2-dicyano-1,2-ethanedithiolate (maleonitriledithiolate, mnt) complexes were measured by means of X-ray photoelectron spectroscopy (XPS), and the energy differences between N1s and S2s, ΔE, were found to be 171.7–172.6 eV throughout the complexes studied. The lowest ΔE value, 171.7 eV, was shown by [Ni(mnt)2]−. The electronic structures of [Ni(mnt)2]− and [Ni(mnt)2]2− were calculated by the discrete variational Xα method. The XPS measurements and the molecular orbital (MO) calculations provide consistent results that the oxidation state of the nickel atom is +2 for both nickel mnt complexes and that the highest occupied MO is 5b3g, which is mainly localized on ligands and which holds an unpaired electron in [Ni(mnt)2]−." @default.
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- W1997627838 date "1981-09-01" @default.
- W1997627838 modified "2023-09-27" @default.
- W1997627838 title "The Electronic Structures of Bis(<i>cis</i>-1,2-dicyano-1,2-ethenedithiolato)nickel Complexes" @default.
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- W1997627838 doi "https://doi.org/10.1246/bcsj.54.2636" @default.
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