FRINK Linked Data Fragments server

Matches in SemOpenAlex for { <https://semopenalex.org/work/W1997661421> ?p ?o ?g. }

• W1997661421 endingPage "23249" @default.
• W1997661421 startingPage "23241" @default.
• W1997661421 abstract "The role of sea-salt aerosol in the sulphur dioxide budget is investigated using a steady state box model. The model simulates, for certain species, the condensation onto, and chemical reactions within, deliquescent sea-salt particles. The chemical reactions are controlled by the pH of the solution, and results show that the presence of gas-phase nitric acid, HNO 3 , and ammonia, NH 3 , can have a significant effect on calculated concentrations of non-sea-salt (nss) sulphate, [nss-SO 4 2 -], formed within the solution. For example, in the case of high [HN 3(g) (100 pptv) the calculated [nss-SO 4 2 -] can be decreased by ∼ 40% after 2 days (with a 75% decrease at HNO 3 concentrations of 1 ppbv). When NH 3 is added, a decrease in calculated [nss-SO 4 2 -] of 20% is observed for 500 pptv NH 3 , 50 pptv HNO 3 . Thus nitric acid is more effective than ammonia. In conditions appropriate for the marine boundary layer (50 pptv of SO 2 , and HNO 3 , and 200 pptv of NH 3 ), nitric acid is still the governing factor, and the [nss-SO 4 2- ], after 2 days, is decreased by approximately 25% compared to the concentration formed when conditions show no HNO 3 or NH 3 . Results also show that comparisons with nss-SO 4 2- observations are nearly 1 order of magnitude lower, with observations giving a [nss-SO 4 2- ]:Na + ratio of 0.01-0.04 compared to predicted values of 0.005 or lower. Other mechanisms of nss-sulphate production may have to be used to explain all the nss-sulphate found in sea-salt aerosol. Although in cases where [SO 2(g) ] is 10-100 pptv the decrease in [nss-SO 4 2 .] is 15-30%, at values of [SO 2(g) ] > 100 pptv the effects of both nitric acid and ammonia on calculated [nss-SO 4 2 .] are small. In a future scenario of increasing NO x (HNO 3 ) emissions and decreasing SO 2 emissions the role of HNO 3 on the global sulphur budget could be very significant." @default.
• W1997661421 created "2016-06-24" @default.
• W1997661421 creator A5068674490 @default.
• W1997661421 creator A5088614401 @default.
• W1997661421 date "1997-10-01" @default.
• W1997661421 modified "2023-10-16" @default.
• W1997661421 title "Sensitivity of sulphur dioxide oxidation in sea salt to nitric acid and ammonia gas phase concentrations" @default.
• W1997661421 cites W1570045084 @default.
• W1997661421 cites W1963658509 @default.
• W1997661421 cites W1976327816 @default.
• W1997661421 cites W1984336016 @default.
• W1997661421 cites W1987234766 @default.
• W1997661421 cites W1993672312 @default.
• W1997661421 cites W2020151793 @default.
• W1997661421 cites W2022991339 @default.
• W1997661421 cites W2034643367 @default.
• W1997661421 cites W2037709506 @default.
• W1997661421 cites W2046136706 @default.
• W1997661421 cites W2046847095 @default.
• W1997661421 cites W2049082872 @default.
• W1997661421 cites W2068441711 @default.
• W1997661421 cites W2086263041 @default.
• W1997661421 cites W2088026022 @default.
• W1997661421 cites W2088283266 @default.
• W1997661421 cites W210583670 @default.
• W1997661421 cites W2108123877 @default.
• W1997661421 cites W2129514998 @default.
• W1997661421 cites W2156151041 @default.
• W1997661421 cites W2173852084 @default.
• W1997661421 cites W4242739573 @default.
• W1997661421 cites W4242968616 @default.
• W1997661421 doi "https://doi.org/10.1029/97jd01621" @default.
• W1997661421 hasPublicationYear "1997" @default.
• W1997661421 type Work @default.
• W1997661421 sameAs 1997661421 @default.
• W1997661421 citedByCount "12" @default.
• W1997661421 crossrefType "journal-article" @default.
• W1997661421 hasAuthorship W1997661421A5068674490 @default.
• W1997661421 hasAuthorship W1997661421A5088614401 @default.
• W1997661421 hasConcept C107872376 @default.
• W1997661421 hasConcept C178790620 @default.
• W1997661421 hasConcept C179104552 @default.
• W1997661421 hasConcept C185592680 @default.
• W1997661421 hasConcept C2776371256 @default.
• W1997661421 hasConcept C2776382133 @default.
• W1997661421 hasConcept C2778504605 @default.
• W1997661421 hasConcept C2778804858 @default.
• W1997661421 hasConcept C2779345167 @default.
• W1997661421 hasConcept C2780447027 @default.
• W1997661421 hasConcept C2780723490 @default.
• W1997661421 hasConcept C3020013744 @default.
• W1997661421 hasConcept C39432304 @default.
• W1997661421 hasConcept C44280652 @default.
• W1997661421 hasConcept C518881349 @default.
• W1997661421 hasConceptScore W1997661421C107872376 @default.
• W1997661421 hasConceptScore W1997661421C178790620 @default.
• W1997661421 hasConceptScore W1997661421C179104552 @default.
• W1997661421 hasConceptScore W1997661421C185592680 @default.
• W1997661421 hasConceptScore W1997661421C2776371256 @default.
• W1997661421 hasConceptScore W1997661421C2776382133 @default.
• W1997661421 hasConceptScore W1997661421C2778504605 @default.
• W1997661421 hasConceptScore W1997661421C2778804858 @default.
• W1997661421 hasConceptScore W1997661421C2779345167 @default.
• W1997661421 hasConceptScore W1997661421C2780447027 @default.
• W1997661421 hasConceptScore W1997661421C2780723490 @default.
• W1997661421 hasConceptScore W1997661421C3020013744 @default.
• W1997661421 hasConceptScore W1997661421C39432304 @default.
• W1997661421 hasConceptScore W1997661421C44280652 @default.
• W1997661421 hasConceptScore W1997661421C518881349 @default.
• W1997661421 hasIssue "D19" @default.
• W1997661421 hasLocation W19976614211 @default.
• W1997661421 hasOpenAccess W1997661421 @default.
• W1997661421 hasPrimaryLocation W19976614211 @default.
• W1997661421 hasRelatedWork W103845754 @default.
• W1997661421 hasRelatedWork W145623635 @default.
• W1997661421 hasRelatedWork W1997661421 @default.
• W1997661421 hasRelatedWork W2031006073 @default.
• W1997661421 hasRelatedWork W2069078107 @default.
• W1997661421 hasRelatedWork W2096382779 @default.
• W1997661421 hasRelatedWork W2116543570 @default.
• W1997661421 hasRelatedWork W2166793237 @default.
• W1997661421 hasRelatedWork W2233329245 @default.
• W1997661421 hasRelatedWork W2357066437 @default.
• W1997661421 hasVolume "102" @default.
• W1997661421 isParatext "false" @default.
• W1997661421 isRetracted "false" @default.
• W1997661421 magId "1997661421" @default.
• W1997661421 workType "article" @default.