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- W1998071310 abstract "The densities of silicon and of silicon containing interstitial Li+ were determined. There is a volume expansion of 4.7×10—24 cm3 per Li+ dissolved in silicon. This expansion is interpreted as arising from the Coulombic repulsion between the Li+ and the partially shielded Si4+ cores. Calculations based on a simple model of the charge distribution in silicon are in accord with this interpretation. The density change accompanying the room temperature deionization and aggregation of the lithium was also measured. During the initial stages of this process, the volume increases linearly by 6.0×10—24 cm3 per lithium transferred from the ionized to the deionized state. This expansion is interpreted as arising from overlap repulsive forces between the Si and aggregates of neutral lithium in neighboring interstitial sites. Considerations based on the size of Li0 in these aggregates and the free energy change for the deionization and aggregation process support this interpretation. A final nonlinear region in the observed volume expansion is interpreted as being due to the precipitation of lithium metal so as to leave itself and the silicon strain free." @default.
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- W1998071310 date "1961-11-01" @default.
- W1998071310 modified "2023-10-18" @default.
- W1998071310 title "Effect of Interstitial Li on the Density of Si" @default.
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- W1998071310 doi "https://doi.org/10.1063/1.1732148" @default.
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