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• W1998085037 abstract "The first example of the palladium-catalyzed exclusive 5-exo-dig hydroarylation of o-alkynyl biaryls has been demonstrated. In contrast to the reported earlier carbocyclizations proceeding via the Friedel-Crafts mechanism, this hydroarylation efficiently proceeds with electron-neutral and electron-deficient arenes, producing fluorene frameworks with defined stereochemistry of the double bond. On the basis of the high reactivity of electron-deficient arenes toward cyclization, high values of inter- and intramolecular kinetic isotope effects, and the exclusive cis-selectivity of cyclization, a mechanism involving a C-H activation motif has been proposed for this transformation." @default.
• W1998085037 created "2016-06-24" @default.
• W1998085037 creator A5003400425 @default.
• W1998085037 creator A5050359844 @default.
• W1998085037 date "2008-03-22" @default.
• W1998085037 modified "2023-10-18" @default.
• W1998085037 title "Exclusive 5-<i>exo-dig</i> Hydroarylation of <i>o</i>-Alkynyl Biaryls Proceeding via C−H Activation Pathway" @default.
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• W1998085037 doi "https://doi.org/10.1021/ja8006534" @default.
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