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• W1998200681 abstract "We report high-resolution x-ray Raman scattering studies of high-order multipole spectra of rare earth excitations (the absorption edge) in nanoparticles of the phosphates LaPO4, CePO4, PrPO4, and NdPO4. We also present corresponding data for La excitations (the edge) in LaPO4. The results are compared with those from calculations by atomic multiplet theory and for the dipole contribution to the La transition from a calculation using time-dependent density functional theory (TDLDA). Agreement with the atomic multiplet calculations for the high-order multiplet spectra is remarkable in the case of the spectra. In contrast, we find that the shallow semicore excitations in LaPO4 manifest a relatively broad band and an apparent quenching of spin-orbit splitting. The more sophisticated TDLDA, which has earlier been found to explain dipolar spectra well in Ba compounds, is less satisfactory here in the case of La." @default.
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• W1998200681 date "2015-04-20" @default.
• W1998200681 modified "2023-10-17" @default.
• W1998200681 title "High-resolution nonresonant x-ray Raman scattering study on rare earth phosphate nanoparticles" @default.
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• W1998200681 doi "https://doi.org/10.1088/1367-2630/17/4/043041" @default.
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