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• W1998620300 abstract "The kinetics of photochlorination of tetrachloroethene in the presence or in the absence of a solvent (CCl4) in which mass transfer from the gas to the liquid phase is followed by fast free-radical reactions initiated with light was studied in a model stirred contactor with a plane liquid interface. Measurements of the gas- and liquid-side mass transfer coefficients were made in the contactor by using Cl2CCl4 and Cl2KJaq systems, respectively. The solubility of chlorine in reaction mixtures and of hexachloroethane in CCl4 and C2Cl4 was also determined. The kinetic parameters of the reaction rate model derived from the study of the photoreaction in a homogeneous system were identified based on experimental results in the gas—liquid system. The validity of the reaction rate model for homogeneous photoreaction in the presence of carbon tetrachloride was confirmed for C2Cl4 concentrations above 2 mol/dm3 in the reaction mixture. Kinetic parameters for homogeneous and heterogeneous systems in the presence of the solvent were compared and discussed." @default.
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• W1998620300 date "1993-07-01" @default.
• W1998620300 modified "2023-09-23" @default.
• W1998620300 title "Kinetics of tetrachloroethene photochlorination" @default.
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• W1998620300 doi "https://doi.org/10.1016/0009-2509(93)81065-4" @default.
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