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• W1999079876 abstract "Abstract In this work, the optical absorption and ESR spectra of mixed conductive lithium borotungstate glasses are measured. The spin density as well as the weight percent of W6+ ions are calculated. The electronic structure of tungsten ions and the network structure of the glasses are analyzed. It is found that both tungsten ions W5+ and W6+ co-exist in the glasses with Li2O content less than 35 mol% and there are predominately W6+ ion in the glasses with Li2O content >35 mol%. The optical absorption caused by W5+ ions decreases with increasing Li2O content and rapidly increases with increasing WO3 content. The spin density, however, anomalously weakens with increasing WO3 content so as to be zero finally in contrast with the optical properties of the glasses. It follows that the increase of WO3 content must lead to the polymerization of tungsten-oxygen polyhedra and therefore, there must exist two electrons with paired spins in the 5d-state of tungsten ions in the larger tungstate clusters." @default.
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• W1999079876 date "1992-09-01" @default.
• W1999079876 modified "2023-09-24" @default.
• W1999079876 title "Optical absorption and ESR spectra of mixed conductive glasses in Li2O-B2O3-WO3 system☆" @default.
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• W1999079876 doi "https://doi.org/10.1016/0167-2738(92)90080-9" @default.
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