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- W1999772024 abstract "Abstract New Raman and i.r. data on CaUO4, including isotopic and solid solutions frequencies, are presented and interpreted with the support of a group theoretical analysis and a normal coordinate treatment. The oxygen atoms only are allowed to move during the four Raman-active modes, all of which have been observed. The vibrational behaviour of the Ca1-xSrxUO4 solid solutions suggests that two of these modes are conveniently described by internal motions of the uranyl group, viz. symmetric stretch (696 cm−1) and librational (340 cm−1) motions. Similarly, solid solution frequencies and 40Ca-44Ca isotopic shifts lead to a satisfactory assignment of the five observed (against six predicted) i.r. frequencies: internal motions of the uranyl ion (696 and 366 cm−1 for the antisymmetric stretching, and bending respectively), translations of the Ca++ ion (305 and 165−1), and translation of the oxygen (435 cm−1). Most of these assignments do not agree with those previously proposed. The non-reproducibility of some i.r. frequencies is also discussed." @default.
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- W1999772024 date "1977-01-01" @default.
- W1999772024 modified "2023-10-18" @default.
- W1999772024 title "Infrared and Raman spectrum of CaUO4: New data and interpretations" @default.
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- W1999772024 doi "https://doi.org/10.1016/0584-8539(77)80074-3" @default.
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