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- W1999881551 abstract "The influence of the ohmic drop on the electrode kinetics controlled by the activation energy has been examined by assuming two prevailing processes and a simple representation of the metal-solution interphase by an electrical dipole. The mathematical formalism has permitted the introduction of the apparent polarization resistance, Rpa, and the form factor H which is essential for a correct use of the linear polarization method. Artificial data, relating to the interval [−20,20]mV, were obtained with reference to the curve described by Ba = 30 mV, Bc = 120 mV and Ic = 0.100 mA cm−2 by searching for the roots of a suitable function with the Newton method at various values of Rs. Other artificial data were generated by considering the same values of Ba and Bc, assuming Rs = 2 Ω and changing the value of Ic. The analysis of both sets of artificial data by the NOLI method was successful and permitted the dependence of the electrochemical parameters on Rs or Ic to be determined quantitatively. The analysis of data concerning Rs = 2 Ω and Ic ranging from 0.1 to 1.0 mA cm−2 stresses the importance of reducing the contribution of the ohmic drop to the electrode potential because Ica takes values greater than the true ones. Examination of some examples concerning artificial and experimental data showed that the form factor is essential for the calculation of the actual value of Ic when its determination is based on the use of Rpa." @default.
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- W1999881551 date "1996-04-01" @default.
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- W1999881551 title "A theoretical study of the influence of the ohmic drop on polarization curves" @default.
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- W1999881551 doi "https://doi.org/10.1016/0010-938x(95)00156-e" @default.
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