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• W1999911962 abstract "Herein, we present the synthesis of a metal–organic framework-based tandem catalyst that contains two distinct catalytic domains. Zn(II)-based IRMOF-9-Irdcppy-NH2 (IRMOF = isoreticular metal–organic framework) has both organocatalytic amine and organometallic Ir(I) groups that were incorporated by both pre- and postsynthetic functionalization methods. The isolated amine and Ir(I) sites of IRMOF-9-Irdcppy-NH2 are shown to be independently catalytically active for performing a Knoevenagel condensation and allylic N-alkylation, respectively. More importantly, IRMOF-9-Irdcppy-NH2 can act as a tandem catalyst for both of these organic transformations in a one-pot reaction, which cannot be achieved efficiently using the combined, homogeneous analogues." @default.
• W1999911962 created "2016-06-24" @default.
• W1999911962 creator A5028132671 @default.
• W1999911962 creator A5088021045 @default.
• W1999911962 date "2015-03-18" @default.
• W1999911962 modified "2023-10-10" @default.
• W1999911962 title "A Bifunctional, Site-Isolated Metal–Organic Framework-Based Tandem Catalyst" @default.
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• W1999911962 doi "https://doi.org/10.1021/ic502316v" @default.
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