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• W2000033790 abstract "Reductive activation of O2 by H2 with rhodium terpyridine complexes in H2O and CH3CN is described and the mechanism is fully elucidated. The rhodium complex extracts electrons from H2 and reductively activates O2 to form a peroxo active intermediate. This intermediate is able to oxidise triphenyl phosphine to triphenyl phosphine oxide. A model system constructed in CH3CN provides isolable analogues of catalytic intermediates in H2O, allowing a detailed look at each step in the catalytic cycle." @default.
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• W2000033790 date "2012-01-01" @default.
• W2000033790 modified "2023-10-11" @default.
• W2000033790 title "Establishing the mechanism of Rh-catalysed activation of O₂by H₂" @default.
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• W2000033790 doi "https://doi.org/10.1039/c1dt11599e" @default.
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