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- W2000058049 abstract "Transition probabilities have been calculated as a function of vibrational and rotational level for the A2Σ+−X2πi system of the hydroxyl molecule. The wavefunctions are obtained from RKR calculations. The electronic transition moment is constructed by adding a small hyperbolic tail at large internuclear distance r (taken from an ab initio calculation) to a linear form at small r; this linear form was validated in earlier studies by laser-excited fluorescence measurements, calculations, and an examination of literature data. The results show, as anticipated, a variation in transition probability with rotatinaal quantum number J, the degree of which varies with vibrational band. The widely used results of Anketell and Learner, based on an inferior form of the transition moment, are accurate to within about 10% for the range J = 0−20 within a given vibrational band, although not from band to band." @default.
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- W2000058049 date "1980-02-01" @default.
- W2000058049 modified "2023-09-27" @default.
- W2000058049 title "Calculated rotational transition probabilities for the A−X system of OH" @default.
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- W2000058049 doi "https://doi.org/10.1016/0022-4073(80)90006-0" @default.
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