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- W2000119838 abstract "In situ Fourier transform infrared (FTIR) extinction spectra of airborne α-NAD microparticles generated by two different methods were recorded in the large coolable aerosol chamber AIDA of Forschungszentrum Karlsruhe. The extinction spectrum of α-NAD crystals obtained by shock freezing of a HNO3/H2O gas mixture could be accurately reproduced using Mie theory with published refractive indices of α-NAD as input. In contrast, Mie theory proved to be inadequate to properly reproduce the infrared extinction spectrum of α-NAD crystals which were formed via homogeneous nucleation of supercooled HNO3/H2O solution droplets, evaporating slowly on a time scale of several hours at about 195 K. Much better agreement between measured and calculated extinction spectra was obtained by T-matrix calculations assuming oblate particles with aspect ratios greater than five. This indicates that strongly aspherical α-NAD crystals are obtained when supercooled nitric acid solution droplets freeze and grow slowly, a process which has been discussed as a potential pathway to the formation of crystalline polar stratospheric cloud (PSC) particles." @default.
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- W2000119838 date "2005-02-23" @default.
- W2000119838 modified "2023-10-14" @default.
- W2000119838 title "Infrared Spectrum of Nitric Acid Dihydrate: Influence of Particle Shape" @default.
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- W2000119838 doi "https://doi.org/10.1021/jp044997u" @default.
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