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- W2000179400 abstract "Abstract CuCl 2 /TiO 2 -based catalysts were examined to investigate the role of copper chloride for the oxidation of gaseous elemental mercury in selective catalytic reduction (SCR) process. CuCl 2 on CuCl 2 /TiO 2 catalyst was decomposed releasing Cl by calcination at high temperatures and restored to its original form by being exposed to gas phase HCl, reversibly. The activity for mercury oxidation was significantly increased with the increase of CuCl 2 loading and HCl concentration. CuCl 2 /TiO 2 catalysts revealed high activity for mercury oxidation even in the absence of HCl. This suggests that mercury oxidation could occur via a Mars–Maessen mechanism by which adsorbed or weakly bound Hg 0 would react with Cl in CuCl 2 that is replenished from gas phase HCl. However, the activity of CuCl 2 -loaded catalysts for NO removal considerably decreased with the increase of temperature above 300–350 °C, which may be due to the ability of CuCl 2 for NH 3 oxidation in SCR reaction." @default.
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- W2000179400 date "2010-08-01" @default.
- W2000179400 modified "2023-10-03" @default.
- W2000179400 title "Oxidation of gaseous elemental mercury by hydrochloric acid over CuCl2/TiO2-based catalysts in SCR process" @default.
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- W2000179400 doi "https://doi.org/10.1016/j.apcatb.2010.06.032" @default.
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