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- W2000218605 abstract "A Monte Carlo (MC) algorithm is presented for the simulation of the time evolution of aggregation processes featuring multiple components, properties, or conservation laws. Instead of using deterministic differential population balance equations, the MC algorithm utilizes a stochastic approach to aggregation kinetics. As a result, exact simulation of spatially independent aggregation processes is possible without the need for numerical approximations. Furthermore, simulations exactly predict all moments of the size and composition distributions of aggregating particles for both nongelling and gelling kernels and extend these results to the postgelation period. The algorithm is shown to require at most O((Ω1Ω2…Ωκ)1/(κ+1)) rate-limiting operations per time step for a κ-component aggregation process featuring Ωi monomers of each component i—a substantial performance improvement over the potential of previous methods. Simulation results are presented for bivariate sum, product, and constant kernels, and for the perikinetic (Brownian) kernel." @default.
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- W2000218605 date "2002-04-01" @default.
- W2000218605 modified "2023-10-09" @default.
- W2000218605 title "A General Algorithm for Exact Simulation of Multicomponent Aggregation Processes" @default.
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- W2000218605 doi "https://doi.org/10.1006/jcph.2002.7017" @default.
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