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- W2000263654 endingPage "4173" @default.
- W2000263654 startingPage "4165" @default.
- W2000263654 abstract "A series of neutral and cationic Ru(II) complexes (1–10), bearing pyridine-based tridentate (′N ͡N ͡N′), pyridine-based bidentate (N ͡N′), and mixed ′N ͡N ͡N′ + N ͡N′ ligands, were synthesized by starting from [RuCl2(DMSO)4] and [RuCl2(p-cymene)]2 precursors. Solid-state structures of mixed-ligand complexes 9 and 10 were determined by single-crystal X-ray diffraction. Both complexes are unusual in that N ͡N′ ligands were spontaneously oxidized in air under base-free conditions to give imine-amine bidentate ligands upon replacement of p-cymene by meridional ′N ͡N ͡N′. The complexes 1–10 were screened for transfer hydrogenation (TH) of aryl ketones with 2-propanol. The highest catalytic activity was obtained with the complexes containing tridentate ′N ͡N ͡N′ and 7, which contain nonsulfonated 2-(aminomethyl)pyridine. However, for complexes 6a–c, containing p-cymene (a facial tridentate ligand), a slower reaction rate was observed." @default.
- W2000263654 created "2016-06-24" @default.
- W2000263654 creator A5051363626 @default.
- W2000263654 creator A5078063665 @default.
- W2000263654 creator A5081453473 @default.
- W2000263654 creator A5083099924 @default.
- W2000263654 creator A5084856181 @default.
- W2000263654 date "2011-07-12" @default.
- W2000263654 modified "2023-10-18" @default.
- W2000263654 title "Synthesis of Ruthenium(II) Complexes Containing Tridentate Triamine (′N ͡N ͡N′) and Bidentate Diamine Ligands (N ͡N′): as Catalysts for Transfer Hydrogenation of Ketones" @default.
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- W2000263654 doi "https://doi.org/10.1021/om200470p" @default.
- W2000263654 hasPublicationYear "2011" @default.