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• W2000286812 abstract "Bathochromic UV–Vis spectral shifts of two hydrophilically N-substituted Michler's ketone derivatives, 4,4′-bis[di(2-hydroxyethyl)amino]benzophenone [MK(OH)4] (1) and 4-(dimethylamino)-4′-[di(2-hydroxyethyl)-amino]benzophenone [MK(OH)2] (3), were measured in 28 solvents of different polarity. For MK(OH)4 and MK(OH)2 in non-polar, dipolar aprotic and hydrogen-bonding solvents, the solvatochromic responses of the two solutes conform exactly to the requirements of the Kamlet-Taft linear solvation free energy model of solvent–solute interactions. The contribution of the hydrogen-bond accepting property of the solvent on the bathochromic band shift of MK(OH)4 and MK(OH)2 increases with increasing number of their OH groups at the N-substituent. The x-ray crystallographic analysis for MK(OH)2 reveals the presence of strong intermolecular hydrogen bonds between the carbonyl oxygen atom and the 2-hydroxyethyl group, which plays a significant role in the colour of the crystals. Copyright © 2001 John Wiley & Sons, Ltd." @default.
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• W2000286812 date "2001-03-05" @default.
• W2000286812 modified "2023-10-11" @default.
• W2000286812 title "Linear solvation energy (LSE) correlations of the solvatochromic response and x-ray structure analysis of hydrophilically<i>N</i>-substituted Michler's ketone derivatives" @default.
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• W2000286812 doi "https://doi.org/10.1002/poc.359" @default.
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