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- W2000291296 endingPage "193" @default.
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- W2000291296 abstract "To contribute solutions to current energy concerns, improvements in the efficiency of dioxygen mediated C-H bond cleavage chemistry, for example, selective oxidation of methane to methanol, could minimize losses in natural gas usage or produce feedstocks for fuels. Oxidative C-H activation is also a component of polysaccharide degradation, potentially affording alternative biofuels from abundant biomass. Thus, an understanding of active-site chemistry in copper monooxygenases, those activating strong C-H bonds is briefly reviewed. Then, recent advances in the synthesis-generation and study of various copper-oxygen intermediates are highlighted. Of special interest are cupric-superoxide, Cu-hydroperoxo and Cu-oxy complexes. Such investigations can contribute to an enhanced future application of C-H oxidation or oxygenation processes using air, as concerning societal energy goals." @default.
- W2000291296 created "2016-06-24" @default.
- W2000291296 creator A5084521304 @default.
- W2000291296 creator A5087301464 @default.
- W2000291296 date "2015-04-01" @default.
- W2000291296 modified "2023-10-03" @default.
- W2000291296 title "Elaboration of copper–oxygen mediated C–H activation chemistry in consideration of future fuel and feedstock generation" @default.
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- W2000291296 doi "https://doi.org/10.1016/j.cbpa.2015.02.014" @default.
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