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- W2000351138 abstract "After a brief introduction to neutron scattering techniques, illustrated with the scattering function for harmonic oscillators, some new aspects of proton dynamics in the KHCO3 crystal are presented. The full scattering function for the proton modes measured on single crystals provides a graphic view of proton dynamics. Vibrational states are fully characterized with three quantum numbers. The effective oscillator mass of 1 amu confirms the decoupling of protons from the lattice. Combining infrared, Raman and inelastic neutron scattering techniques, the double minimum potential for the transfer of a single proton along hydrogen bonds is totally determined. Elastic neutron scattering techniques probe dynamics in the fully degenerate ground state. Quantum entanglement arising from normal coordinates gives rise to quantum interference. With diffraction techniques, the dynamical structure arising from large-scale quantum coherence is observed as ridges of intensity, well separated from Bragg's peaks. The vibrational wave function in the ground state must be regarded as a superposition of non-factorable macroscopic wave function." @default.
- W2000351138 created "2016-06-24" @default.
- W2000351138 creator A5048990977 @default.
- W2000351138 date "2004-08-01" @default.
- W2000351138 modified "2023-09-25" @default.
- W2000351138 title "Proton dynamics in an extended array of hydrogen bonds: normal coordinates, proton transfer and macroscopic quantum entanglement in the ground state" @default.
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- W2000351138 doi "https://doi.org/10.1016/j.molstruc.2004.01.008" @default.
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