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- W2000352746 abstract "Fenestranes are regarded as a particularly challenging synthetic targets, and only few syntheses have been reported in the recent past. These rare compounds of synthetic and theoretical interest are a class of tetracyclic skeletons, defined as doubly a,a′-bridged spiroalkanes. The reported results are focused on the synthesis of new and original [4.6.4.6]fenestradienes 3a−f and [4.6.4.6]fenestrenes 4a−e. Our approach implies the formation of this tetracyclic structure by a reaction cascade, based on consecutive transformations starting from the trienyne 1a−f: an initial soft hydrogenation using a P-2 Nickel catalyst at room temperature, followed by a conrotatory 8p electrocyclization and a disrotatory 6p electrocyclization and a final oxidation. Several examples of this type of new compounds are described in this Communication." @default.
- W2000352746 created "2016-06-24" @default.
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- W2000352746 date "2008-03-19" @default.
- W2000352746 modified "2023-10-10" @default.
- W2000352746 title "Synthesis of [4.6.4.6]Fenestradienes and [4.6.4.6]Fenestrenes Based on an 8π−6π-Cyclization-Oxidation Cascade" @default.
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- W2000352746 doi "https://doi.org/10.1021/ja800691c" @default.
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