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- W2000372728 abstract "The relaxation of the $1P$ to $1S$ electronic states of CdSe semiconductor nanocrystals is followed by infrared pump-probe spectroscopy. Fast (1 ps) and slow (>200 ps) components are observed. Using different capping molecules to control the hole states, we show how the intraband relaxation slows down as the hole is in a shallow trap, a deep trap, or a charge-separated complex, providing strong support for an electron-hole Auger coupling. The slow component corresponds to an energy relaxation rate orders of magnitude slower than in bulk systems. It may be the first indication of the phonon bottleneck effect long expected in strongly confined quantum dots." @default.
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- W2000372728 date "1999-07-15" @default.
- W2000372728 modified "2023-09-23" @default.
- W2000372728 title "Intraband relaxation in CdSe quantum dots" @default.
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- W2000372728 doi "https://doi.org/10.1103/physrevb.60.r2181" @default.
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