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- W2000373428 abstract "This communication describes the design and execution of a novel approach to forming chiral lactones via C−H bond activation. The strategy features an unprecedented enantioselective Rh-catalyzed hydroacylation of carbon−oxygen double bonds. Representative keto-aldehydes (derived from salicylaldehyde) undergo cyclization with complete regioselectivity to afford seven-membered lactones in great enantiomeric excess (≥99% ee). The basicity of the phosphine ligand is shown to play a critical role in promoting hydroacylation over competitive decarbonylation." @default.
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- W2000373428 date "2008-02-16" @default.
- W2000373428 modified "2023-10-18" @default.
- W2000373428 title "Rh-Catalyzed Carbonyl Hydroacylation: An Enantioselective Approach to Lactones" @default.
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- W2000373428 doi "https://doi.org/10.1021/ja7109025" @default.
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