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- W2000437074 abstract "The gas-phase ion-molecule reactions between the nucleogenic methyl cations, generated by the β-decay of the tritiated methane, and hexamethyldisilazane were studied by the radiochromatographic method. The appearance of the observed labelled products is rationalized assuming formation of the two major types of the intermediate ion-neutral complexes, i.e., methylated and protonated disilazane. Some observed products contain silylium groups whose structure are different from those of precursors. Isomerization and the ethene expulsion of the silylium groups, which are the characteristic reactions of free silylium cations, are suggested to occur during the lifetime of the intermediate ion-neutral complexes. Triton transfer from CT3+ to disilazane produces tritiated methylene. Products of insertion of CT2 into NH and CH bonds of substrate are also observed." @default.
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- W2000437074 date "1997-12-01" @default.
- W2000437074 modified "2023-09-22" @default.
- W2000437074 title "Radiochemical study of the reactions between the methyl cation and hexamethyldisilazane" @default.
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- W2000437074 doi "https://doi.org/10.1016/s0022-328x(97)00458-0" @default.
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