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- W2000477522 abstract "A model of the electron-stimulated desorption of physisorbed species is proposed in which the excited-state surface potential is due to a chemical rather than image force acting on the adsorbed particle after the initial electron excitation is completed. The equilibrium positions of the excited- and the ground-state potentials nearly coincide and desorption is a purely quantum-mechanical effect. A one-dimensional model is systematically derived from the three-dimensional theory. The oscillatory structure of the resulting kinetic-energy distributions of the desorbing species is predicted in certain cases. It is demonstrated that, unlike in the commonly accepted Antoniewicz model, both the kinetic-energy distributions of the desorbing neutral particles and the total desorption yield calculated in the present model are consistent with the experimental data for Ar and ${mathrm{N}}_{2}$O physisorbed on Ru(001)." @default.
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- W2000477522 date "1991-04-01" @default.
- W2000477522 modified "2023-09-27" @default.
- W2000477522 title "Theory of electron-stimulated desorption of physisorbed species through a strongly bonding excited state" @default.
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- W2000477522 doi "https://doi.org/10.1103/physrevb.43.7487" @default.
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