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- W2000481164 abstract "Abstract An expression for calculating the molar concentration ratio of CO/CO 2 produced on a burning carbon surface is presented. Three reactions on the surface of the carbon particle burning in air are considered: (a) C + O 2 → CO 2 , (b) C + 1/2O 2 → CO, and (c) C + CO 2 → 2CO; whereas in the gas phase surrounding the particle there is the homogeneous reaction: CO + 1/2O 2 → CO 2 . The molar concentration ratio of primary product CO to CO 2 formed by reactions a and b on the carbon surface is CO/CO 2 = g co( b ) / g co2( a ) . M co2 / M co , where g co( b ) is the mass flux of CO by reaction b on the carbon surface, g co2( a ) is the mass flux of CO 2 by reaction a on the carbon surface, whereas M co and M co2 are the molar weights of CO and CO 2 , respectively. To find this ratio, the burning rate and temperature are measured. Based on experiments and the solution of a set of equations for a large carbon particle (3-mm diameter), the oxygen content on the surface of the burning particle is calculated. This gives the reaction order and frequency factor of the reactions C + 1/2O 2 → CO and C + O 2 → O 2 . The surface ratio of CO/CO 2 can be obtained, provided the surface oxygen concentration is known. The advantage of this method is that the burning rate and temperature can be accurately measured. Good agreement between experiment and calculation shows the proposed expression for CO/CO 2 to be an improvement on previous ones." @default.
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- W2000481164 date "1996-11-01" @default.
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- W2000481164 title "The ratio CO/CO2 of oxidation on a burning carbon surface" @default.
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- W2000481164 doi "https://doi.org/10.1016/s0010-2180(96)00071-5" @default.
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